Document Type

Thesis

Date of Degree Completion

Summer 1973

Degree Name

Master of Science (MS)

Department

Chemistry

Committee Chair

Richard Wayne Hasbrouck

Second Committee Member

J. Jones

Third Committee Member

W. Emken

Abstract

The preparation and characterization of select cyclic ethynyl carbinols is presented as a preliminary step for a more detailed investigation of the Rupe rearrangement. The objective of the research work was to attempt to predict abnormal chemical behavior from spectral characteristics of each of the cyclic ethynyl carbinols. Preparation of the starting carbinols was accomplished by a modified Grignard synthesis. Nuclear magnetic resonance spectroscopy, infrared spectroscopy and mass spectroscopy were used for characterization of each new carbinol prepared. The spectral data available from the characterization work were then used to establish a correlation between ring size and appropriate absorption maxima. Analogies from the literature were used for the spectral correlation work since spectral data for all members of the series studies are currently unavailable. The analogs chosen were less substituted appropriate compounds. Subjects to the extent that analogous absorption maxima hold, definite trends in maxima were found to parallel ring size.

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Chemistry Commons

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